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By Joshua Jortner, Raphael D. Levine, Stuart Alan Rice

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17 for the respective temperatures. The surprisals calculated from all three of these models thus indicate a preference for vibrational energy in promoting the reaction. Work is now progressing on a temperature analysis of both the steady-state and laserexcited reactions in order to provide further evidence. ” The diffusion cloud method can thus be seen to be a potentially useful technique for studying the reactions of laser-excited polyatomic molecules. Since the reactant sodium is monitored, the same technique can be used for a large number of molecular reactants.

60,4568 (1974). R. Bersohn and H. Horowitz, J. Chem. , 63, 48 (1975). F. Ackerman and E. Miescher, J. Mol. Spectry, 31, 400 (1969). 0. Benoist d'Azy, R. Lopez Delgado, and A. Tramer, Chem. , 9, 327 (1975). A. B. Callear, M. J. Pilling, and I. W. M. Smith, Trans. ,64, 2296 (1968). J. 0. Hirschfelder, C. E. Curtiss, and R. B. Bird, Molecular Theory of Guses and Liquids, Wiley, New York, 1964. H. Okabe, J. Am. Chem. , 93, 7095 (1971). APPLICATION TO NITRIC OXIDE FLUORESCENCE QUENCHING 41 40. (a) G.

ASSCHER 20 attainment of high peak powers while avoiding optical damage to cell windows and associated optics by keeping average power as low as possible. In kinetic studies laser-pumped dye lasers offer both spectral tunability and resolution on the one hand, and good time resolution on the other hand. With typical available dye laser systems (pumped by a nitrogen or a Nd-YAG laser) pulse duration and energy are s and l o p 3J, respectively. Using the data of the above example, about 10" photons are absorbed per laser pulse, creating 5 X lo9 excited molecules.

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